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Electrical Pumping of Perovskite Diodes: Toward Stimulated …

We achieve a strong electrical pumping (ELQE 0.8% at 840 A cm −2) and optically excited ASE (with a threshold of 180 µJ cm −2) simultaneously in a single …

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Strain regulates the photovoltaic performance of thick-film …

The diffusion coefficient was extracted from the TRS measurements under a pump energy of 2.30, 1.90, and 1.65 eV. ... Subsequently, based on this perovskite platform, we demonstrated that lattice ...

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Real-Time Tracking of Hot Carrier Injection at the Interface of …

In the present study, the electron injection dynamics at the interface of the organic–inorganic hybrid perovskite, formamidinium lead bromide (FAPbBr 3), and the organic electron acceptor, IEICO-4F (the chemical structure is shown in Figure S1a and b), are investigated by using fs-mid-IR spectroscopy to follow the ν(C≡N) and ν(C=O ...

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Perovskite solar cells: an emerging photovoltaic technology

The base technology for perovskite solar cells is solid-state sensitized solar cells that are based on dye-sensitized Gratzel solar cells. In 1991, O''Regan and Gratzel developed a low-cost photoelectrochemical solar cell based on high surface area nanocrystalline TiO 2 film sensitized with molecular dye [10].Although the PCE of dye …

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Controlled Synthesis of Lead-Free Double Perovskite Colloidal ...

Although lead-free double perovskites such as Cs 2 AgBiBr 6 have been widely explored, they still remain a daunting challenge for the controlled synthesis of lead-free double perovskite nanocrystals with highly tunable morphology and band structure. Here, we report the controlled synthesis of lead-free double perovskite colloidal …

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Electron tunneling at the molecularly thin 2D perovskite and …

Insulating molecular layers on the basal plane of 2D perovskite is a major bottleneck for charge injection that limiting device performance. Here, the authors show that plane-contacted graphene ...

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Inorganic Halide Perovskite Quantum Dots: A Versatile …

highlighted. Finally, inorganic perovskite QDs as an active layer in the application of transistors and memory devices will be discussed, which will be followed by a perspective on the future developments of perovskite QD electronics. 2 Basic Physical Properties of Inorganic Perovskite QDs 2.1 Lattice Structure of Inorganic Perovskite QDs

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Focus on perovskite emitters in blue light-emitting diodes

Blue perovskite light-emitting diodes (PeLEDs) are essential in pixels of perovskite displays, while their progress lags far behind their red and green counterparts. Here, we focus on recent ...

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Double Layer Composite Electrode Strategy for Efficient Perovskite ...

Perovskite solar cells (PSCs) have become the representatives of next generation of photovoltaics; nevertheless, their stability is insufficient for large scale deployment, particularly the reverse bias stability. Here, we propose a transparent conducting oxide (TCO) and low-cost metal composite electrode to improve the stability …

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From optical pumping to electrical pumping: the threshold ...

144| Mater.Hori., 2023, 10, 1446€1453 This journal is † The Royal Society of Chemistry 2023 Citethis:Mater. Horiz.,2023, 10,1 446 From optical pumping to electrical pumping: the threshold overestimation in metal halide perovskites† Jiajun Qin, ab Yang Tang,a Jia Zhang,b Tangyao Shen,a Max Karlsson,b Tiankai Zhang,b Weidong Cai,b Lei Shi,*a Wei …

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Perovskite solar cells: Stability lies at interfaces

Perovskite solar cells are developing fast but their lifetimes must be extended. Now, large-area printed perovskite solar modules have been shown to be stable for more than 10,000 hours under ...

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Facet-selective growth of halide perovskite/2D semiconductor van …

The introduced monolayer semiconductor not only endows a robustly facet-selective epitaxial growth of perovskite with well-defined planar configuration required for …

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Frontiers | A Perspective on Perovskite Solar Cells: Emergence ...

The state-of-the-art perovskite-on-silicon tandem solar cell has achieved a PCE of 29.52% in Oxford PV on approximately 30 × 30 cm 2 device area (Al-Ashouri et al., 2020). More recently, the all-perovskite tandem solar cell with a certified efficiency of 26.4% has also been reported by (Lin et al., 2022).

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Interface engineering of highly efficient perovskite solar cells

Organic-inorganic hybrid materials, particularly the perovskite family, have shown great promise for use in field-effect transistors, light-emitting diodes, sensors, and photodetectors for more than a decade ().Recently, the power conversion efficiency (PCE) of lead halide perovskite (CH 3 NH 3 PbX 3, X = Cl, Br, I)–based thin film photovoltaic …

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Quasi-2D Dion-Jacobson phase perovskites as a promising …

In summary, we present quasi-2D D-J phase perovskite thin films as a promising platform for stable and high-performance perovskite lasers. The brominated …

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Reconfigurable perovskite nickelate electronics for artificial ...

Reconfigurable devices offer the ability to program electronic circuits on demand. In this work, we demonstrated on-demand creation of artificial neurons, synapses, and memory capacitors in post-fabricated perovskite NdNiO 3 devices that can be simply reconfigured for a specific purpose by single-shot electric pulses. The sensitivity of …

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Halide Perovskite Artificial Solids as a New Platform to …

we introduce artificiallattices made of lead halide perovskite nanocubes as a new platform to simulate and investigate the physics of correlated quantum materials. We demonstrate …

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Electrical Pumping of Perovskite Diodes: Toward Stimulated …

a) Current density (J) and outcoupled photon flux density of our perovskite diode as a function of voltage (V) in DC or AC.(inset: the image of the pixel used for the measurement) b) Measured ELQE and c) EL spectrum at each J.d) Electrical circuit used for pulsed measurement, having a load resistance (R L) between a fixed input voltage (V 1) …

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Halide Perovskite Artificial Solids as a New Platform to Simulate ...

The development of quantum simulators, artificial platforms where the predictions of many-body theories of correlated quantum materials can be tested in a controllable and tunable way, is one of the main challenges of condensed matter physics. Here we introduce artificial lattices made of lead halide perovskite nanocubes as a new platform to simulate and …

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Electron injection and defect passivation for high-efficiency ...

Herein, we demonstrate that the ETL in p-MPSCs extracts electrons from perovskite in mesopores at the mesoscale through three-dimensional (3D) injection at the bulk interface to constrain the long-distance diffusion of electrons toward the back electrode.

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Fabrication of Perovskite/Si periodic microwire arrays via micro …

We explore a micro-pump strategy for injecting perovskite materials into Si micro-channels, allowing fabrication of many perovskite micro-wires (MWs) to form inside the regularly …

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Electron injection and defect passivation for high-efficiency ...

Printable mesoscopic PSCs (p-MPSCs) are an alternative platform that does not use HTLs or metal electrodes. In p-MPSCs, the perovskite is infiltrated into the scaffold of mesoporous TiO 2 (mp-TiO 2)/mesoporous ZrO 2 (mp-ZrO 2)/mesoporous carbon (mp-C) (2, 3).

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Resonant perovskite solar cells with extended band edge

a Theoretical Shockley-Queisser (S-Q) limit efficiency (black line) and record cell efficiency of GaAs 4, perovskite single crystals (perovskite SC) 14, and thin films (FAPbI 3 8, MAPbI 3 41, and ...

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Overcoming Shockley-Queisser limit using halide perovskite platform ...

In this paper, we first dissect the origin of the limit, and then, by using the emerging perovskite as the platform, we list several potential pathways (i.e., hot carrier, multi-exciton generation, intermediate band gap, and ferroelectricity that have been newly discovered or can be introduced in the perovskite) to the roadmap of exceeding the ...

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Perovskite materials as superior and powerful platforms for …

Abstract. In order to meet the continuously growing demand for clean energy, a plethora of advanced materials have been exploited for energy storage …

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Room-temperature-processed perovskite solar cells surpassing …

The photoactive FAPbI 3 cubic structure is thermodynamically metastable and only exists at temperatures above 117°C (390 K), as shown in Figure 1 A. 13, 14 At RT, the metastable cubic perovskite with a higher Gibbs free energy can spontaneously transform back into the energetically stable photoinactive hexagonal phase. 13, 14 Tuning …

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Perovskite enables high performance vanadium redox flow battery

1. Introduction. Nowadays, the demand for energy is increasing due to fast social development, which enhances the dependance of green energy sources including solar, wind and tidal energy [1], [2], [3], [4].The solution to address the imbalance between supply and demand is to develop energy storage and transfer by rechargeable battery …

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Perovskite Quantum Dots in Solar Cells

With porphyrin-bridging, a stable 0D–2D perovskite capping layer were formed. Ultimately, compared with pure perovskite and CsPbBr 3 PQDs modification, the PCE is higher with CsPbBr 3 PQDs modified treated by ZnPy-NH 3 Br. The bulk perovskite presents more durable stability after ligand-exchange, too.

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Bandgap-universal passivation enables stable perovskite solar …

Because multijunction perovskite-on-silicon and all-perovskite tandem cells usually use thermally evaporated C 60 as an ETL, to demonstrate the compatibility of our passivation treatment, we fabricated Cs 17 Br 23 with an evaporated C 60 and BCP ETL stack and obtained an enhancement of V OC from 1.21 V for the Cs 17 Br 23 reference …

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Advances in the Application of Perovskite Materials

Nowadays, the soar of photovoltaic performance of perovskite solar cells has set off a fever in the study of metal halide perovskite materials. The excellent optoelectronic properties and defect tolerance feature allow metal halide perovskite to be employed in a wide variety of applications. This article provides a holistic review over the …

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